By Ruijun Hou
This thesis deals novel equipment for catalyst and approach layout for the selective hydrogenation of acetylene and 1,3-butadiene. the writer predicts the houses of supported Pd–Ni bimetallic catalysts utilizing density practical thought (DFT) calculations and temperature-programmed desorption (TPD). the wonderful correlation among version surfaces and supported catalysts demonstrates the feasibility of designing powerful bimetallic catalysts for selective hydrogenation reactions. the writer additionally proposes a style for designing non-precious steel catalysts to switch useful metals. she alters the method of selective hydrogenation of acetylene by means of coupling the selective adsorption to the selective hydrogenation within the liquid section, due to which the ethylene selectivity is vastly enhanced and warmth move is significantly more advantageous. finally, through studying the mechanism of liquid-phase hydrogenation, the writer proposes a multi-stage slurry mattress reactor for commercial applications.<
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Catalytic and Process Study of the Selective Hydrogenation of Acetylene and 1,3-Butadiene (Springer Theses) by Ruijun Hou
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